- William as Paddington Bear
- Fireman Sam as Mr. Brown
- Penny Morris as Mrs. Brown
- Pingi as Judy Brown
- Pingu as Jonathan Brown
- Joshua Jones as David Russell
- Lars the Little Polar Bear as Mrs. Bird
- Big Ears as Mr. Gruber
- Norman Price as Mr. Curry
- Miss Hubbard as Madame Helenka
- Daphne as Aunt Lucy
- Sly and Gobbo as Burglars
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