- Captain America/Steve Rogers as Tinky Winky
- Iron Man/Tony Stark as Tigers
- Black Widow/Natasha Romanoff as Laa Laa
- Hawkeye/Clint Barton as Frogs
- Winter Soldier/Bucky Barnes as The Scary Lion
- Black Panther/T'Challa as Giraffes
- Baron Helmut Zemo as The Dog
- Thunderbolt Ross as Elephants
- Ant-Man/Scott Lang as The Puppet Scotsman
- Scarlet Witch/Wanda Maximoff as Little Bo Peep
- Spider-Man/Peter Parker as Dipsy
- Christine Everhart as Po
- Peggy Carter as The Sun
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