- Alvin Seville (Alvin and the Chipmunks) as Larry the Cucumber as Buccaneer Larry
- Theodore Seville (Alvin and the Chipmunks) as Mr. Lunt as Pirate Lunt
- Simon Seville (Alvin and the Chipmunks) as Pa Grape as Captain Pa
Chapter 1: Introduction
- Simon: Ahoy there, maties! Captain Simon here! Welcome aboard the ship of the Pirates Who Don't Do Anything!
- Theodore: Nothing.
- Alvin: Zilch.
- Theodore: Nada.
- Simon: Not so fast, ya lazies! Today, we're doing a little something.
- Alvin: (irritated) Not again!
- Theodore: We did something yesterday!
- Simon: Huh? All you did was order Chinese!
- Theodore: Hey, it's hard to say moo goo guy pan! Whoop, I did it again. I'm beat.
- Alvin: Here, have a won-ton.
Chapter 2: "Endangered Love"
Chapter 3: "The Dance of Sheen Estevez"
Chapter 4: "Sheen's High Silk Hat"
Chapter 5: Technical Difficulties?!?
Chapter 6: "The Water Buffalo Song"
Chapter 7: "The Yodeling Veterinarian of the Alps"
Chapter 8: "The Song of the Minions"
Chapter 9: "Do the Moo Shoo"
Chapter 10: "His Cheeseburger"
Chapter 11: "Love My Lips"
Chapter 12: Something Fishy?
Chapter 13: The Confession
Chapter 14: "The Pirates Who Don't Do Anything"
Chapter 15: "The Hairbrush Song"
- Simon: Well, that's it! The great Silly Song Countdown is complete!
- Alvin: Thanks for voting, everyone! You guys are great!
- Theodore: Yeah, thanks!
- (Alvin walks up to the camera)
Alvin: Kung pao squid?