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- Marlon as Captain Scarlet/Paul Metcalfe
- Robbie as Captain Blue/Adam Svenson
- Buggles as Lieutenant Green/Seymour Griffiths
- Tiger Lily as Destiny Angel/Juliette Pontoin
- Jeffries as Symphony Angel/Karen Wainwright
- Tabs as Rhapsody Angel/Dianne Simms
- Sims as Melody Angel/Magnolia Jones
- Ransome as Harmony Angel/Chan Kwan
- Kenneth as Captain Brown
- Dr Kawashima as Colonel White/Charles Gray
- Baron Silas Greenback as Captain Black/Conrad Turner