- Brainy Smurf as Peter Pan
- Smurfette as Wendy
- Clumsy Smurf as John
- Nat Smurfling as Michael
- Grouchy Smurf as Captain Hook
- Duncan (from Thomas and Friends) as Mr. Smee
- Emily (from Thomas and Friends) as Mary Darling
- Tuffy Smurf as George Darling
- and more
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