- Homer as Mr. Potts
- Marge as Truly Scumptious
- Bart as Jeremy
- Lisa as Jemima
- Grandpa Abe as Grandpa
- Ned Flanders as The Toy Maker
- Principal Skinner as Lord Scrumptious
- Wendy Testaburger (from South Park) as Chitty Chitty Bang Bang (Wendy Testaburger and Chitty Chitty Bang Bang are both Beautiful)
- Sideshow Bob as Baron Bomburst
- Edna Krabappel as Baroness Bomburst
- Mr. Burns as The Child Catcher
- Nelson Muntz and Jimbo Jones as Herman and Sherman
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