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- Diesel as Horrid Henry
- Antione (from Sonic) as Perfect Peter
- Sir Topham Hatt as Dad
- Thomas as Goody-Goody Gordon
- Lady as Gorgeous Gurinder
- Toad as Brainy Brian
- Diesel 10 as Stuck-Up Steve
- Daisy as Moody Margret (Not Molly! Molly is thoughtful and kind, Moody Margaret is bossy and mean)
- Mavis as Sour Susan (Not Lady! Lady is nice, Sour Susan is mean)
- Molly as Lazy Linda
- Rosie as Prissy Polly
- Gordon as Mr. Mossy (Not James!)